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dc.contributor.author肖梅玲
dc.contributor.author祝建兵
dc.contributor.author刘长鹏
dc.contributor.author葛君杰
dc.contributor.author邢巍
dc.contributor.authorXIAO Mei-ling
dc.contributor.authorZHU Jian-bing
dc.contributor.authorLIU Chang-peng
dc.contributor.authorGE Jun-jie
dc.contributor.authorXING Wei
dc.date.accessioned2016-05-09T07:32:20Z
dc.date.available2016-05-09T07:32:20Z
dc.date.issued2016-05-03
dc.identifier.citation电化学,2016,22(2):101-112.
dc.identifier.issn1006-3471
dc.identifier.urihttp://dx.doi.org/10.13208/j.electrochem.151152
dc.identifier.urihttps://dspace.xmu.edu.cn/handle/2288/98304
dc.description.abstract燃料电池中广泛使用的铂基催化剂价格昂贵、储量低、容易失活,因此亟待开发廉价、高效非铂催化剂. 过渡金属(Fe、Co、Ni等)/杂原子共掺杂催化剂、杂原子掺杂(N、P、S、F等)碳材料以及碳材料包覆过渡金属复合物是目前发现的几类性能优异的非贵金属氧还原催化剂. 其中碳材料包覆过渡金属催化剂作为一类新型的高性能催化剂,对其研究还有待深入. 本文主要阐述了国内外在包覆型非贵金属氧还原催化剂方面的研究进展,从合成,性能,机理等方面对该类催化剂进行了总结,力求助益于该类催化剂的发展.
dc.description.abstractPlatinum-based materials, the state-of-the-art catalysts for fuel cells, suffer from prohibitive costs, limited resources and insufficient durability. Accordingly, tremendous efforts were made in searching for efficient, durable and inexpensive alternatives to precious-metal electrocatalysts for the oxygen reduction reaction (ORR). Transition-metals (Fe, Co)/nitrogen co-doped hybrids, heteroatom (N, P, S, F, et al) doped carbons and composites with transition-metals encapsulated in graphitic layers are reported as the most efficient non-precious metal ORR catalysts. Among the various non-precious metal ORR catalysts, transition-metals encased in graphitic layer catalysts are a novel type of catalysts for ORR with high activity and durability, and thus, the in-depth researches are highly desirable. Here, we present the recent research progress in transition-metals encased catalysts from the aspects of synthesis, activity and catalytic mechanism, in an effort to promote the developments of these catalysts.
dc.description.sponsorship科技部973项目(No. 2012CB215500)、国家自然科学基金项目(No. 21373199,No. 21433003)、中国科学院先导专项(No. XDA09030104)、吉林省科技发展项目(No. 20130206068GX,No. 20140203012SF,No. 20102204)和吉林省自然科学基金项目(No. 20150101066JC)资助
dc.language.isozh
dc.publisher厦门大学《电化学》编辑部
dc.relation.ispartofseries燃料电池电催化和催化剂近期研究专辑(重庆大学 魏子栋教授主编)
dc.relation.ispartofseriesSpecial issue of Electrocatalyst and Electrocatalysis in Fuel Cells(Editor: Professor Wei Zi-dong)
dc.source.urihttp://electrochem.xmu.edu.cn/CN/abstract/abstract10261.shtml
dc.subject氧还原反应
dc.subject过渡金属包覆
dc.subject非贵金属催化剂
dc.subjectoxygen reduction reaction
dc.subjecttransition-metals encased
dc.subjectnon-precious metal catalysts
dc.title包覆型非贵金属氧还原催化剂的研究进展
dc.title.alternativeRecent Progress in Non-Precious Metal Oxygen Reduction Reaction Catalysts with an Encapsulation Structure
dc.typeArticle
dc.description.note作者联系地址:1. 中国科学院长春应用化学研究所,电分析国家重点实验室,吉林 长春 130022;2. 中国科学院长春应用化学研究所,先进化学电源实验室,吉林 长春 130022
dc.description.noteAuthor's Address: 1. State Key Laboratory of Electroanalytical Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, China; 2. Laboratory of Advanced Power Sources, Changchun Institute of Applied Chemistry, Changchun 130022, China
dc.description.note通讯作者E-mail:xingwei@ciac.ac.cn


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